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Making tracks

The magnitude of the effect of anthropogenic aerosols on the formation of clouds is an important unknown about how humans are affecting climate. Studies of stratocumulus cloud tracks that are formed by ship exhaust have been used to estimate the radiative impact of this process, but Glassmeier et al. now show that this approach overestimates the cooling effect of aerosol addition by up to 200%. These findings underscore the need to quantify stratocumulus cloud responses to anthropogenic aerosols to understand the climate system.
Science, this issue p. 485

Abstract

The effect of anthropogenic aerosol on the reflectivity of stratocumulus cloud decks through changes in cloud amount is a major uncertainty in climate projections. In frequently occurring nonprecipitating stratocumulus, cloud amount can decrease through aerosol-enhanced cloud-top mixing. The climatological relevance of this effect is debated because ship exhaust only marginally reduces stratocumulus amount. By comparing detailed numerical simulations with satellite analyses, we show that ship-track studies cannot be generalized to estimate the climatological forcing of anthropogenic aerosol. The ship track–derived sensitivity of the radiative effect of nonprecipitating stratocumulus to aerosol overestimates their cooling effect by up to 200%. The offsetting warming effect of decreasing stratocumulus amount needs to be taken into account if we are to constrain the cloud-mediated radiative forcing of anthropogenic aerosol.
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Supplementary Material

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Supplementary Text
Figs. S1 to S6
Tables S1 to S4
References (4145)

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References and Notes

1
G. L. Stephens, J. Li, M. Wild, C. A. Clayson, N. Loeb, S. Kato, T. L’Ecuyer, P. W. Stackhouse Jr.., M. Lebsock, T. Andrews, An update on Earth’s energy balance in light of the latest global observations. Nat. Geosci. 5, 691–696 (2012).
2
T. S. L’Ecuyer, Y. Hang, A. V. Matus, Z. Wang, Reassessing the effect of cloud type on Earth’s energy balance in the age of active spaceborne observations. Part I: Top of atmosphere and surface. J. Clim. 32, 6197–6217 (2019).
3
O. Boucher et al., Climate Change 2013: The Physical Science Basis. Working Group I Contribution to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, T. F. Stocker et al., Eds. (Intergovernmental Panel on Climate Change, 2013).
4
N. Bellouin, J. Quaas, E. Gryspeerdt, S. Kinne, P. Stier, D. Watson-Parris, O. Boucher, K. S. Carslaw, M. Christensen, A.-L. Daniau, J.-L. Dufresne, G. Feingold, S. Fiedler, P. Forster, A. Gettelman, J. M. Haywood, U. Lohmann, F. Malavelle, T. Mauritsen, D. T. McCoy, G. Myhre, J. Mülmenstädt, D. Neubauer, A. Possner, M. Rugenstein, Y. Sato, M. Schulz, S. E. Schwartz, O. Sourdeval, T. Storelvmo, V. Toll, D. Winker, B. Stevens, Bounding global aerosol radiative forcing of climate change. Rev. Geophys. 58, RG000660 (2020).
5
S. Twomey, Pollution and the planetary albedo. Atmos. Environ. 8, 1251–1256 (1974).
6
B. A. Albrecht, Aerosols, cloud microphysics, and fractional cloudiness. Science 245, 1227–1230 (1989).
7
S. Wang, Q. Wang, G. Feingold, Turbulence, condensation, and liquid water transport in numerically simulated nonprecipitating stratocumulus clouds. J. Atmos. Sci. 60, 262–278 (2003).
8
A. S. Ackerman, M. P. Kirkpatrick, D. E. Stevens, O. B. Toon, The impact of humidity above stratiform clouds on indirect aerosol climate forcing. Nature 432, 1014–1017 (2004).
9
C. S. Bretherton, P. N. Blossey, J. Uchida, Cloud droplet sedimentation, entrainment efficiency, and subtropical stratocumulus albedo. Geophys. Res. Lett. 34, L03813 (2007).
10
J. D. Small, P. Y. Chuang, G. Feingold, H. Jiang, Can aerosol decrease cloud lifetime? Geophys. Res. Lett. 36, L16806 (2009).
11
F. Hoffmann, G. Feingold, Entrainment and mixing in stratocumulus: Effects of a new explicit subgrid-scale scheme for large-eddy simulations with particle-based microphysics. J. Atmos. Sci. 76, 1955–1973 (2019).
12
B. Stevens, G. Feingold, Untangling aerosol effects on clouds and precipitation in a buffered system. Nature 461, 607–613 (2009).
13
J. Mülmenstädt, G. Feingold, The radiative forcing of aerosol–cloud interactions in liquid clouds: Wrestling and embracing uncertainty. Curr. Clim. Change Rep. 4, 23–40 (2018).
14
M. W. Christensen, G. L. Stephens, Microphysical and macrophysical responses of marine stratocumulus polluted by underlying ships: Evidence of cloud deepening. J. Geophys. Res. 116, D03201 (2011).
15
E. Gryspeerdt, T. Goren, O. Sourdeval, J. Quaas, J. Mülmenstädt, S. Dipu, C. Unglaub, A. Gettelman, M. Christensen, Constraining the aerosol influence on cloud liquid water path. Atmos. Chem. Phys. 19, 5331–5347 (2019).
16
V. Toll, M. Christensen, J. Quaas, N. Bellouin, Weak average liquid-cloud-water response to anthropogenic aerosols. Nature 572, 51–55 (2019).
17
M. S. Diamond, H. M. Director, R. Eastman, A. Possner, R. Wood, Substantial cloud brightening from shipping in subtropical low clouds. AGU Advances 1, e2019AV000111 (2020).
18
S. Platnick, S. Twomey, Determining the susceptibility of cloud albedo to changes in droplet concentration with the Advanced Very High Resolution Radiometer. J. Appl. Meteorol. 33, 334–347 (1994).
19
R. Boers, R. M. Mitchell, Absorption feedback in stratocumulus clouds Influence on cloud top albedo. Tellus A 46, 229–241 (1994).
20
J. A. Coakley Jr., C. D. Walsh, Limits to the aerosol indirect radiative effect derived from observations of ship tracks. J. Atmos. Sci. 59, 668–680 (2002).
21
A. A. Hill, G. Feingold, H. Jiang, The influence of entrainment and mixing assumption on aerosol–cloud interactions in marine stratocumulus. J. Atmos. Sci. 66, 1450–1464 (2009).
22
S. S. Lee, J. E. Penner, S. M. Saleeby, Aerosol effects on liquid‐water path of thin stratocumulus clouds. J. Geophys. Res. 114, D07204 (2009).
23
H. Wang, P. J. Rasch, G. Feingold, Manipulating marine stratocumulus cloud amount and albedo: A process-modelling study of aerosol-cloud-precipitation interactions in response to injection of cloud condensation nuclei. Atmos. Chem. Phys. 11, 4237–4249 (2011).
24
D. Rosenfeld, Y. Zhu, M. Wang, Y. Zheng, T. Goren, S. Yu, Aerosol-driven droplet concentrations dominate coverage and water of oceanic low-level clouds. Science 363, eaav0566 (2019).
25
A. Possner, R. Eastman, F. Bender, F. Glassmeier, Deconvolution of boundary layer depth and aerosol constraints on cloud water path in subtropical stratocumulus decks. Atmos. Chem. Phys. 20, 3609–3621 (2020).
26
F. Glassmeier, G. Feingold, Network approach to patterns in stratocumulus clouds. Proc. Natl. Acad. Sci. U.S.A. 114, 10578–10583 (2017).
27
D. C. Leon, Z. Wang, D. Liu, Climatology of drizzle in marine boundary layer clouds based on 1 year of data from CloudSat and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO). J. Geophys. Res. 113, D00A14 (2008).
28
H. Xue, G. Feingold, B. Stevens, Aerosol effects on clouds, precipitation, and the organization of shallow cumulus convection. J. Atmos. Sci. 65, 392–406 (2008).
29
Y.-C. Chen, M. W. Christensen, G. L. Stephens, J. H. Seinfeld, Satellite-based estimate of global aerosol–cloud radiative forcing by marine warm clouds. Nat. Geosci. 7, 643–646 (2014).
30
F. A.-M. Bender, L. Frey, D. T. McCoy, D. P. Grosvenor, J. K. Mohrmann, Assessment of aerosol–cloud–radiation correlations in satellite observations, climate models and reanalysis. Clim. Dyn. 52, 4371–4392 (2019).
31
F. Hoffmann, F. Glassmeier, T. Yamaguchi, G. Feingold, Liquid water path steady states in stratocumulus: Insights from process-level emulation and mixed-layer theory. J. Atmos. Sci. 77, 2203–2215 (2020).
32
W. H. Schubert, J. S. Wakefield, E. J. Steiner, S. K. Cox, Marine stratocumulus convection. Part II: Horizontally inhomogeneous solutions. J. Atmos. Sci. 36, 1308–1324 (1979).
33
I. Sandu, B. Stevens, On the factors modulating the stratocumulus to cumulus transitions. J. Atmos. Sci. 68, 1865–1881 (2011).
34
C. S. Bretherton, J. Uchida, T. N. Blossey, Slow manifolds and multiple equilibria in stratocumulus-capped boundary layers. J. Adv. Model. Earth Syst. 2, 20 (2010).
35
R. Wood, Stratocumulus clouds. Mon. Weather Rev. 140, 2373–2423 (2012).
36
M. W. Christensen, K. Suzuki, B. Zambri, G. L. Stephens, Ship track observations of a reduced shortwave aerosol indirect effect in mixed‐phase clouds. Geophys. Res. Lett. 41, 6970–6977 (2014).
37
P. A. Durkee, R. E. Chartier, A. Brown, E. J. Trehubenko, S. D. Rogerson, C. Skupniewicz, K. E. Nielsen, S. Platnick, M. D. King, Composite ship track characteristics. J. Atmos. Sci. 57, 2542–2553 (2000).
38
H. Wang, G. Feingold, Modeling mesoscale cellular structures and drizzle in marine stratocumulus. Part II: The microphysics and dynamics of the boundary region between open and closed cells. J. Atmos. Sci. 66, 3257–3275 (2009).
39
Y.-C. Chen, M. W. Christensen, D. J. Diner, M. J. Garay, Aerosol-cloud interactions in ship tracks using Terra MODIS/MISR. J. Geophys. Res. Atmos. 120, 2819–2833 (2014).
40
R. Wood, T. Ackerman, P. Rasch, K. Wanser, Could geoengineering research help answer one of the biggest questions in climate science? Earths Futur. 5, 659–663 (2017).
41
F. Glassmeier, F. Hoffmann, J. S. Johnson, T. Yamaguchi, K. S. Carslaw, G. Feingold, An emulator approach to stratocumulus susceptibility. Atmos. Chem. Phys. 19, 10191–10203 (2019).
42
G. Feingold, A. McComiskey, T. Yamaguchi, J. S. Johnson, K. S. Carslaw, K. S. Schmidt, New approaches to quantifying aerosol influence on the cloud radiative effect. Proc. Natl. Acad. Sci. U.S.A. 113, 5812–5819 (2016).
43
D. Rosenfeld, G. Gutman, Retrieving microphysical properties near the tops of potential rain clouds by multispectral analysis of AVHRR data. Atmos. Res. 34, 259–283 (1994).
44
T. Michibata, K. Suzuki, Y. Sato, T. Takemura, The source of discrepancies in aerosol-cloud-precipitation interactions between GCM and A-Train retrievals. Atmos. Chem. Phys. 16, 15413–15424 (2016).
45
R. Eastman, R. Wood, C. S. Bretherton, Time scales of clouds and cloud-controlling variables in subtropical stratocumulus from a Lagrangian perspective. J. Atmos. Sci. 73, 3079–3091 (2016).

Information & Authors

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Published In

Science
Volume 371 | Issue 6528
29 January 2021

Submission history

Received: 23 June 2020
Accepted: 22 December 2020
Published in print: 29 January 2021

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Acknowledgments

F.G. thanks A. Possner and T. Goren for helpful discussions about the interpretation of satellite literature. M. Khairoutdinov graciously provided the System for Atmospheric Modeling (SAM) model. The University of Wyoming, Department of Atmospheric Science, is acknowledged for archiving the radiosonde data. We thank three anonymous reviewers for their helpful comments. Funding: F.G. acknowledges support from The Branco Weiss Fellowship – Society in Science, administered by the ETH Zürich, and from a Veni grant of the Dutch Research Council (NWO). F.H. held a visiting fellowship of the Cooperative Institute for Research in Environmental Sciences (CIRES) at the University of Colorado Boulder, and the NOAA Earth System Research Laboratory, and is supported by the German Research Foundation under grant HO 6588/1-1. J.S.J. and K.S.C. were supported by the Natural Environment Research Council (NERC) under grant NE/I020059/1 (ACID-PRUF) and the UK-China Research and Innovation Partnership Fund through the Met Office Climate Science for Service Partnership (CSSP) China as part of the Newton Fund. K.S.C. is currently a Royal Society Wolfson Research Merit Award holder. This research was partially supported by the Office of Biological and Environmental Research of the U.S. Department of Energy Atmospheric System Research Program Interagency Agreement DE-SC0016275 and by an Earth’s Radiation Budget grant, NOAA CPO Climate & CI #03-01-07-001. Author contributions: F.G., G.F., and F.H. conceived the study; F.G. developed the emulator with support from J.S.J. and K.S.C.; T.Y. performed the simulations. All authors contributed to the final product. Competing interests: All authors declare that they have no competing interests. Data and materials availability: Simulation data are available from https://esrl.noaa.gov/csl/groups/csl9/datasets/data/cloud_phys/2020-Glassmeier-etal/. Radiosonde data can be acccessed at http://www.weather.uwyo.edu/upperair/sounding.html.

Authors

Affiliations

Department of Geoscience and Remote Sensing, Delft University of Technology, P.O. Box 5048, 2600 GA Delft, Netherlands.
Department of Environmental Sciences, Wageningen University, P.O. Box 47, 6700 AA Wageningen, Netherlands.
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA.
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA.
NOAA Chemical Sciences Laboratory, 325 Broadway, Boulder, CO 80305, USA.
Institut für Meteorologie, Ludwig-Maximilians-Universität, Theresienstrasse 37, 80333 München, Germany.
School of Earth and Environment, University of Leeds, Woodhouse Lane, Leeds LS2 9JT, UK.
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA.
NOAA Chemical Sciences Laboratory, 325 Broadway, Boulder, CO 80305, USA.
School of Earth and Environment, University of Leeds, Woodhouse Lane, Leeds LS2 9JT, UK.
NOAA Chemical Sciences Laboratory, 325 Broadway, Boulder, CO 80305, USA.

Funding Information

NOAA Research: CI #03-01-07-001
Royal Society: Wolfson Research Merit Award
The Branco Weiss Fellowship:
CIRES, University of Colorado:

Notes

*Corresponding author. Email: [email protected]

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