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Differential Lead Retention in Zircons: Implications for Nuclear Waste Containment

Science16 Apr 1982Vol 216, Issue 4543pp. 296-298DOI: 10.1126/science.216.4543.296

Abstract

An innovative ultrasensitive technique was used for lead isotopic analysis of individual zircons extracted from granite core samples at depths of 960, 2170, 2900, 3930, and 4310 meters. The results show that lead, a relatively mobile element compared to the nuclear waste-related actinides uranium and thorium, has been highly retained at elevated temperatures (105° to 313°C) under conditions relevant to the burial of synthetic rock waste containers in deep granite holes.

References

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Published In

Science
Volume 216 | Issue 4543
16 April 1982

Submission history

Received: 3 November 1981
Published in print: 16 April 1982

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Authors

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Robert V. Gentry
Chemistry Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830
Thomas J. Sworski
Chemistry Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830
Henry S. McKown
Analytical Chemistry Division, Oak Ridge National Laboratory
David H. Smith
Analytical Chemistry Division, Oak Ridge National Laboratory
R. E. Eby
Analytical Chemistry Division, Oak Ridge National Laboratory
W. H. Christie
Analytical Chemistry Division, Oak Ridge National Laboratory

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Cited by
  1. Alpha-Decay—Induced Fracturing in Zircon: The Transition from the Crystalline to the Metamict State, Science, 236, 4808, (1556-1559), (1987)./doi/10.1126/science.236.4808.1556
    Abstract
  2. Response: Lead Retention in Zircons, Science, 223, 4638, (835-835), (1984)./doi/10.1126/science.223.4638.835-b
    Abstract
  3. Lead Retention in Zircons, Science, 223, 4638, (835-835), (1984)./doi/10.1126/science.223.4638.835-a
    Abstract
  4. Response: Lead Retention in Zircons, Science, 223, 4638, (835-835), (1984)./doi/10.1126/science.223.4638.835.b
    Abstract
  5. Lead Retention in Zircons, Science, 223, 4638, (835-835), (1984)./doi/10.1126/science.223.4638.835.a
    Abstract
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