Origin of Nucleosynthetic Isotope Heterogeneity in the Solar Protoplanetary Disk
Abstract
Stable-isotope variations exist among inner solar system solids, planets, and asteroids, but their importance is not understood. We report correlated, mass-independent variations of titanium-46 and titanium-50 in bulk analyses of these materials. Because titanium-46 and titanium-50 have different nucleosynthetic origins, this correlation suggests that the presolar dust inherited from the protosolar molecular cloud was well mixed when the oldest solar system solids formed, but requires a subsequent process imparting isotopic variability at the planetary scale. We infer that thermal processing of molecular cloud material, probably associated with volatile-element depletions in the inner solar system, resulted in selective destruction of thermally unstable, isotopically anomalous presolar components, producing residual isotopic heterogeneity. This implies that terrestrial planets accreted from thermally processed solids with nonsolar isotopic compositions.
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References and Notes
1
Isotope anomalies are deviations in the stable-isotope composition of an element compared to that of the Earth.
2
J.-L. Birck, Rev. Mineral. Geochem.55, 25 (2004).
3
A. Trinquier, J.-L. Birck, C. J. Allègre, Astrophys. J.655, 1179 (2007).
4
R. Andreasen, M. Sharma, Astrophys. J.655, 874 (2007).
5
J. N. Goswami, K. K. Marhas, M. Chaussidon, M. Gounelle, B. S. Meyer, in Chondrites and the Protoplanetary Disk, A. N. Krot, E. R. D. Scott, B. Reipurth, Eds. (Astrophysical Society of the Pacific, San Francisco, CA, 2005), pp. 485–514.
6
Chondrite meteorites are undifferentiated stony meteorites composed of CAIs, Fe-Mg-silicates spherules called chondrules, and a fine-grained volatile-rich matrix.
7
G. J. MacPherson, A. M. Davis, E. K. Zinner, Meteoritics30, 365 (1995).
8
M. Bizzarro, J. A. Baker, H. Haack, Nature431, 275 (2004).
9
K. Thrane, M. Bizzarro, J. A. Baker, Astrophys. J.646, L159 (2006).
10
J. N. Connelly, Y. Amelin, A. N. Krot, M. Bizzarro, Astrophys. J.675, L121 (2008).
11
D. D. Clayton, Handbook of Isotopes in the Cosmos: Hydrogen to Gallium (Cambridge Univ. Press, Cambridge, UK, 2003).
12
F. R. Niederer, D. A. Papanastassiou, G. J. Wasserburg, Geochim. Cosmochim. Acta45, 1017 (1981).
13
S. Niemeyer, G. W. Lugmair, Earth Planet. Sci. Lett.53, 211 (1981).
14
F. R. Niederer, D. A. Papanastassiou, G. J. Wasserburg, Geochim. Cosmochim. Acta49, 835 (1985).
15
I. Leya, M. Schönbächler, U. Wiechert, U. Krähenbühl, A. N. Halliday, Earth Planet. Sci. Lett.266, 233 (2008).
16
T. R. Ireland, Geochim. Cosmochim. Acta52, 2827 (1988).
17
E. Zinneret al., Geochim. Cosmochim. Acta71, 4786 (2007).
18
Materials and methods are available as supporting online material (SOM) at Science Online.
19
H. Palme, A. Jones, in Treatise on Geochemistry, H. D. Holland, K. K. Turekian, Eds., Vol. 1, Meteorites, Comets and Planets, A. M. Davis, Ed. (Elsevier-Pergamon, Oxford, 2003), pp. 41–61.
20
M. Rotaru, J.-L. Birck, C. J. Allègre, Nature358, 465 (1992).
21
G. R. Huss, A. P. Meshik, J. B. Smith, C. M. Hohenberg, Geochim. Cosmochim. Acta67, 4823 (2003).
22
P. A. Blandet al., Proc. Natl. Acad. Sci. U.S.A.102, 13755 (2005).
23
A. Trinquier, J.-L. Birck, C. J. Allègre, C. Göpel, D. Ulfbeck, Geochim. Cosmochim. Acta72, 5146 (2008).
24
O. Bogdanovski, D. A. Papanastassiou, G. J. Wasserburg, Lunar Planet. Sci.33, 1802 (2002).
25
Financial support for this project was provided by the Danish National Research Foundation, the Danish Natural Science Research Council, and the University of Copenhagen's Programme of Excellence. We thank J. Connelly, G. Huss, H. Haack, F. Richter, R. Mendybaev, and B. Meyer for discussion.
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Science
Volume 324 | Issue 5925
17 April 2009
17 April 2009
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American Association for the Advancement of Science.
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Received: 7 November 2008
Accepted: 5 March 2009
Published in print: 17 April 2009
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